https://dx.doi.org/10.1103/PhysRevLett.49.1857">
 

Title

Microcluster Growth: Transition from Successive Monomer Addition to Coagulation

Abstract

The transition in cluster growth from succesive monomer absorption to cluster coalescence has been observed for CO2 condensed in a supersonic beam under high pressure. A model which considers all cluster-cluster reactions achieves good qualitative agreement with the measured size distributions of the clusters. This is the first attempt to fit an experimental cluster spectrum from a first-principles model.

Department

Physics

Publication Date

12-20-1982

Journal Title

Physical Reviw Letters

Publisher

APS Physics

Digital Object Identifier (DOI)

https://dx.doi.org/10.1103/PhysRevLett.49.1857

Document Type

Article

Rights

©1982 American Physical Society

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